点击次数：

影响因子：5.2

DOI码：10.1039/D6TC00118A

发表刊物：Journal of Materials Chemistry C

摘要：In recent years, transition metal phosphorus trichalcogenides have been successfully applied on multiple occasions in the field of photoelectrochemical (PEC) photodetection. In this work, high-quality SnPS3 crystals were synthesized via the chemical vapor transport method and then exfoliated via the liquid-phase exfoliation method to be utilized as active materials in PEC-type photodetectors. The device exhibited an excellent self-powered response and a broadband detection range from 400 nm to 900 nm in an acidic environment. Under simulated sunlight illumination, it achieved a photocurrent density of 31.2 µA cm−2, a responsivity of 195 µA W−1, and rise and decay times of 75 and 91 ms, respectively. The best photoelectric response performance appeared under 400 nm light excitation, with a photocurrent density and responsivity of 11.04 µA cm−2 and 175.19 µA W−1, respectively. Furthermore, after approximately 6200 s of a long-term cycling test and 66 days of an air stability test, the detector's photocurrent density retention rates were 89.23% and 81.05%, respectively. This work implies the significant potential of SnPS3 for being used in the field of self-powered broadband photodetection.

论文类型：期刊论文

文献类型：J

卷号：14

期号：0

页面范围：7550-7560

是否译文：否

收录刊物：SCI

发布期刊链接：https://pubs.rsc.org/en/content/articlelanding/2026/tc/d6tc00118a/unauth

第一作者：Chengzheng Ye

通讯作者：Xin Zhao

通讯作者：Jiaming Song

合写作者：Zhuo Wang

合写作者：Guoshuai Ban

合写作者：Xin Wang

合写作者：Pengxiang Ning

合写作者：Erli Zhang

合写作者：Dihang Wu

合写作者：Yuliang Song

合写作者：Ruxin Liu

合写作者：Peng Hu

合写作者：Yang Jiao

合写作者：Haibo Fan

合写作者：Feng Teng